A study of the barrier properties of polyethylene coated with nanocellulose/magnetite composite film

Nenad Đorđević; Aleksandar D Marinković; Jasmina B Nikolić; Saša Ž Drmanić; Milica Rančić; Danijela V Brković; Petar S Uskoković

doi:10.2298/JSC151217019D

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Published: Jun 28, 2016

DOI: https://doi.org/10.2298/JSC151217019D

Keywords:

hybrid materials composites inorganic filler polycaprolactone packaging material

Nenad Đorđević

Department of Graphic Engineering, Faculty of Technology and Metallurgy, University of Belgrade, Karnegijeva 4, 11120 Belgrade

Aleksandar D Marinković

Department of Organic Chemistry, Faculty of Technology and Metallurgy, University of Belgrade, Karnegijeva 4, 11120 Belgrade

Jasmina B Nikolić

Department of Organic Chemistry, Faculty of Technology and Metallurgy, University of Belgrade, Karnegijeva 4, 11120 Belgrade

Saša Ž Drmanić

Department of Organic Chemistry, Faculty of Technology and Metallurgy, University of Belgrade, Karnegijeva 4, 11120 Belgrade

Milica Rančić

Faculty of Forestry, University of Belgrade, Kneza Višeslava 1, 11030 Belgrade

Danijela V Brković

Innovation Center, Faculty of Technology and Metallurgy, University of Belgrade, Karnegijeva 4, 11120 Belgrade

Petar S Uskoković

Department of Graphic Engineering, Faculty of Technology and Metallurgy, University of Belgrade, Karnegijeva 4, 11120 Belgrade

Abstract

The morphological, thermal and barrier properties of low-density polyethylene/polycaprolactone-modified nanocellulose hybrid materials were investigated in this paper. Nanonocelulose/magnetite (NC-Fe₃O₄) nanocomposite and maleic acid functionalized NC/magnetite (NCMA-Fe₃O₄) nanocomposite were prepared and used as filler at various concentrations (5, 10 and 15 wt. %) in polycaprolactone (PCL) layer. PE was coated with PCL/NC/magnetite layer. The addition of the filler did not unfavorably affect the inherent properties of the polymer, especially its barrier properties. Oxygen permeation measurements show that the oxygen barrier properties of magnetite enriched PCL film were improved due to chemical activity of added material. The highest level of barrier capacity was observed for PE samples coated with PCL based composite with NCMA-Fe₃O₄micro/-nanofiller, which implies the significant contribution of nanocellulose surface modification with maleic anhydride residue to improved barrier properties.

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[1]

N. Đorđević, “A study of the barrier properties of polyethylene coated with nanocellulose/magnetite composite film”, J. Serb. Chem. Soc., vol. 81, no. 5, pp. 589–605, Jun. 2016.

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Vol. 81 No. 5 (2016)

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Materials

Authors retain copyright and grant the journal right of first publication with the work simultaneously licensed under a Creative Commons Attribution license 4.0 that allows others to share the work with an acknowledgement of the work's authorship and initial publication in this journal.

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